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The dielectric constant dependence on the reaction rate of monochloroacetate with thiosulphate ions.
Author(s):
1. Fahimuddin: Chemistry Department, University of Karachi, Karachi, Pakistan
2. Iqbal Hussain: Chemistry Department, University of Karachi, Karachi, Pakistan
Abstract:
Studies on the reaction rate between sodium monochloroacetate and sodium thiosulphate at 25' and at various concentrations of the reacting ions and various dielectric constant ? with acetone-water mixtures showed that the specific rate constant (k) increased with the dielectric constant. A comparison of the experimental values of the radii of the transient species for single sphere and double sphere models r≠. and rAB ) respectively (obtained from the linear plots of log ko and 1/?) with the theoretical values led to the conclusion that the transient species could best be described by the "SINGLE SPHERE" model for the reaction under consideration. Electrostatic and non-electrostatic contributions to the changes in the free energy of activation (Gand ?G ≠n.e.s ) in the formation of transient species were also evaluated.
Page(s): 91-93
DOI: DOI not available
Published: Journal: Pakistan Journal of Scientific and Industrial Research, Volume: 30, Issue: 2, Year: 1987
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